The first thing I noticed is that by twisting the line until it self-coils into a tight spiral doesn't work very well, since the tight coil doesn't have much room to stretch out and retract like a spring. What I did was twist the line to the point just before it tries to coil up on itself and then wrap it around something to give the coil some diameter.
I used a hex key just because it was metal (so it wouldn't melt in the oven), had a nice diameter, and was within reach. I then used alligator clips to hold the line in place. I then annealed it in the oven at around 360 F for 30 minutes.
Check out the video to see it in action (sorry about the noisy hair dryer)
Well this was extremely interesting to see, although it almost behaves more like a "tendon" than actual muscle.